• Amino

    EC 5. Isomerases

    EC 5. Isomerases
    EC 5.1 Racemases and Epimerases
    EC 5.1.1 Acting on Amino Acids and Derivatives

    EC 5.1.1.1 alanine racemase
    EC 5.1.1.2 methionine racemase
    EC 5.1.1.3 glutamate racemase
    EC 5.1.1.4 proline racemase
    EC 5.1.1.5 lysine racemase
    EC 5.1.1.6 threonine racemase
    EC 5.1.1.7 diaminopimelate epimerase
    EC 5.1.1.8 4-hydroxyproline epimerase
    EC 5.1.1.9 arginine racemase
    EC 5.1.1.10 amino-acid racemase
    EC 5.1.1.11 phenylalanine racemase (ATP-hydrolysing)
    EC 5.1.1.12 ornithine racemase
    EC 5.1.1.13 aspartate racemase
    EC 5.1.1.14 nocardicin-A epimerase
    EC 5.1.1.15 2-aminohexano-6-lactam racemase
    EC 5.1.1.16 protein-serine epimerase
    EC 5.1.1.17 isopenicillin-N epimerase
    EC 5.1.1.18 serine racemase

    EC 5.1.2 Acting on Hydroxy Acids and Derivatives

    EC 5.1.2.1 lactate racemase
    EC 5.1.2.2 mandelate racemase
    EC 5.1.2.3 3-hydroxybutyryl-CoA epimerase
    EC 5.1.2.4 acetoin racemase
    EC 5.1.2.5 tartrate epimerase
    EC 5.1.2.6 isocitrate epimerase

    EC 5.1.3 Acting on Carbohydrates and Derivatives

    EC 5.1.3.1 ribulose-phosphate 3-epimerase
    EC 5.1.3.2 UDP-glucose 4-epimerase
    EC 5.1.3.3 aldose 1-epimerase
    EC 5.1.3.4 L-ribulose-5-phosphate 4-epimerase
    EC 5.1.3.5 UDP-arabinose 4-epimerase
    EC 5.1.3.6 UDP-glucuronate 4-epimerase
    EC 5.1.3.7 UDP-N-acetylglucosamine 4-epimerase
    EC 5.1.3.8 N-acylglucosamine 2-epimerase
    EC 5.1.3.9 N-acylglucosamine-6-phosphate 2-epimerase
    EC 5.1.3.10 CDP-paratose 2-epimerase
    EC 5.1.3.11 cellobiose epimerase
    EC 5.1.3.12 UDP-glucuronate 5′-epimerase
    EC 5.1.3.13 dTDP-4-dehydrorhamnose 3,5-epimerase
    EC 5.1.3.14 UDP-N-acetylglucosamine 2-epimerase
    EC 5.1.3.15 glucose-6-phosphate 1-epimerase
    EC 5.1.3.16 UDP-glucosamine 4-epimerase
    EC 5.1.3.17 heparosan-N-sulfate-glucuronate 5-epimerase
    EC 5.1.3.18 GDP-mannose 3,5-epimerase
    EC 5.1.3.19 chondroitin-glucuronate 5-epimerase
    EC 5.1.3.20 ADP-glyceromanno-heptose 6-epimerase
    EC 5.1.3.21 maltose epimerase
    EC 5.1.3.22 L-ribulose-5-phosphate 3-epimerase
    EC 5.1.3.23 UDP-2,3-diacetamido-2,3-dideoxyglucuronic acid 2-epimerase

    EC 5.1.99 Acting on Other Compounds

    EC 5.1.99.1 methylmalonyl-CoA epimerase
    EC 5.1.99.2 16-hydroxysteroid epimerase
    EC 5.1.99.3 allantoin racemase
    EC 5.1.99.4 α-methylacyl-CoA racemase
    EC 5.1.99.5 hydantoin racemase

    EC 5.2 cis-trans-Isomerases

    EC 5.2.1.1 maleate isomerase
    EC 5.2.1.2 maleylacetoacetate isomerase
    EC 5.2.1.3 retinal isomerase
    EC 5.2.1.4 maleylpyruvate isomerase
    EC 5.2.1.5 linoleate isomerase
    EC 5.2.1.6 furylfuramide isomerase
    EC 5.2.1.7 retinol isomerase
    EC 5.2.1.8 peptidylprolyl isomerase
    EC 5.2.1.9 farnesol 2-isomerase
    EC 5.2.1.10 2-chloro-4-carboxymethylenebut-2-en-1,4-olide isomerase
    EC 5.2.1.11 deleted entry

    EC 5.3 Intramolecular Oxidoreductases

    EC 5.3.1 Interconverting Aldoses and Ketoses

    EC 5.3.1.1 triose-phosphate isomerase
    EC 5.3.1.2 deleted
    EC 5.3.1.3 arabinose isomerase
    EC 5.3.1.4 L-arabinose isomerase
    EC 5.3.1.5 xylose isomerase
    EC 5.3.1.6 ribose-5-phosphate isomerase
    EC 5.3.1.7 mannose isomerase
    EC 5.3.1.8 mannose-6-phosphate isomerase
    EC 5.3.1.9 glucose-6-phosphate isomerase
    EC 5.3.1.10 now EC 3.5.99.6
    EC 5.3.1.11 deleted
    EC 5.3.1.12 glucuronate isomerase
    EC 5.3.1.13 arabinose-5-phosphate isomerase
    EC 5.3.1.14 L-rhamnose isomerase
    EC 5.3.1.15 D-lyxose ketol-isomerase
    EC 5.3.1.16 1-(5-phosphoribosyl)-5-[(5-phosphoribosylamino)methylideneamino]imidazole-4-carboxamide isomerase
    EC 5.3.1.17 4-deoxy-L-threo-5-hexosulose-uronate ketol-isomerase
    EC 5.3.1.18 deleted
    EC 5.3.1.19 now EC 2.6.1.16
    EC 5.3.1.20 ribose isomerase
    EC 5.3.1.21 corticosteroid side-chain-isomerase
    EC 5.3.1.22 hydroxypyruvate isomerase
    EC 5.3.1.23 5-methylthioribose-1-phosphate isomerase
    EC 5.3.1.24 phosphoribosylanthranilate isomerase
    EC 5.3.1.25 L-fucose isomerase
    EC 5.3.1.26 galactose-6-phosphate isomerase
    EC 5.3.1.27 6-phospho-3-hexuloisomerase
    EC 5.3.1.28 D-sedoheptulose 7-phosphate isomerase

    EC 5.3.2 Interconverting Keto- and Enol-Groups

    EC 5.3.2.1 phenylpyruvate tautomerase
    EC 5.3.2.2 oxaloacetate tautomerase

    EC 5.3.3 Transposing C=C Bonds

    EC 5.3.3.1 steroid Δ-isomerase
    EC 5.3.3.2 isopentenyl-diphosphate Δ-isomerase
    EC 5.3.3.3 vinylacetyl-CoA Δ-isomerase
    EC 5.3.3.4 muconolactone Δ-isomerase
    EC 5.3.3.5 cholestenol Δ-isomerase
    EC 5.3.3.6 methylitaconate Δ-isomerase
    EC 5.3.3.7 aconitate Δ-isomerase
    EC 5.3.3.8 dodecenoyl-CoA Δ-isomerase
    EC 5.3.3.9 prostaglandin-A1 .................More Read....

    AMINO ACID ASSAY

    AMINO ACID ASSAY

    BY NINHYDRIN COLORIMETRIC METHOD

    Prepared by

    Nam Sun Wang

    Department of Chemical & Biomolecular Engineering

    University of Maryland

    College Park, MD 20742-2111

    ENCH485



    Method

    The reaction between alpha-amino acid and ninhydrin involved in the development of color are described by the following five mechanistic steps:

      alpha-amino acid + ninhydrin ---> reduced ninhydrin + alpha-amino acid + H2O
    
      alpha-amino acid + H2O ---> alpha-keto acid +NH3
    
      alpha-keto acid + NH3 ---> aldehyde + CO2

    Step (1) is an oxidative deamination reaction that removes two hydrogen from the alpha-amino acid to yield an alpha-imino acid. Simultaneously, the original ninhydrin is reduced and loses an oxygen atom with the formation of a water molecule. In Step (2), the NH group in the alpha-imino acid is rapidly hydrolyzed to form an alpha-keto acid with the production of an ammonia molecule. This alpha-keto acid further undergoes decarboxylation reaction of Step (3) under a heated condition to form an aldehyde that has one less carbon atom than the original amino acid. A carbon dioxide molecule is produced here. These first three steps produce the reduced ninhydrin and ammonia that are required for the production of color in the last two Steps (4) and (5). The overall reaction for the above reactions is simply (slightly inaccurately) expressed in Reaction (6) as follows:

    alpha-amino acid + 2 ninhydrin ---> CO2 + aldehyde + final complex(BlUE) + 3H2O

    In summary, ninhydrin, which is originally yellow, reacts with amino acid and turns deep purple. It is this purple color that is detected in this method.Ninhydrin will react with a free alpha-amino group, NH2-C-COOH. This group is contained in all amino acids, peptides, or proteins. Whereas, the decarboxylation reaction will proceed for a free amino acid, it will not happen for peptides and proteins. Thus, theoretically only amino acids will lead to the color development. However, one should always check out the possible interference from peptides and proteins by performing blank tests especially when such solutions are readily available. For example, one can simply add the ninhydrin reagent to a solution of only proteins and see if there is any color development. There is no excuse for failing to perform such a vital test when the sample mixture contains both proteins and amino acids. There are also reports that chemical compounds other than amino acids also yield positive results.

    This test can be used routinely for the detection of glycine in the absence of other interfering species. Although this is a fast and sensitive test for the presence of alpha-amino acids, because of the nonselectivity, it cannot be used to analyze the relative individual contents of a mixture of different amino acids. Furthermore, the color intensity developed is dependent on the type of amino acid. Finally, it does not react with tertiary or aromatic amines.

    Note that since ninhydrin is a strong oxidizing agent, proper caution should be exercised in handling this compound. It is especially potent at the elevated temperature under which the reaction is carried out. The ninhydrin reagent will stain the skin blue and cannot be immediately washed off completely if it comes in contact with the skin. However, as in any other stain on the skin, the color will gradually rub off after about a day.


    List of Reagents and Instruments

    A. Equipment

      Test tubes
      Pipets
      Spectrophotometer

    B. Reagents

      Ninhydrin Reagent Solution

        Ninhydrin: 0.35 g
        Add ethanol to: 100 ml (See Note 1.)

    Procedures

      Add 1 ml of the ninhydrin solution to 5 ml of sample. Cover the test tube with a piece of paraffin film to avoid the loss of solvent due to evaporation. A capped test tube can also be used instead.
      With gentle stirring, react at 80-100ºC for 4-7 minutes. (How would one find out the amount of time needed to ensure a complete reaction?) If a large heated water bath is used for the entire class and if there is no good provision for holding the test tube in the hot water bath, the test tube may be held with a piece of wire and hang on the side of the water container. A clamp usually does not work too well.
      After cooling to room temperature in a cold water bath, record the absorbance with a
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    Absorbance Assay (280 nm)

    Absorbance Assay (280 nm)

    Considerations for use

    Absorbance assays are fast and convenient, since no additional reagents or incubations are required. No protein standard need be prepared. The assay does not consume the protein. The relationship of absorbance to protein concentration is linear. Because different proteins and nucleic acids have widely varying absorption characteristics there may be considerable error, especially for unknowns or protein mixtures. Any non-protein component of the solution that absorbs ultraviolet light will intefere with the assay. Cell and tissue fractionation samples often contain insoluble or colored components that interfere. The most common use for the absorbance assay is to monitor fractions from chromatography columns, or any time a quick estimation is needed and error in protein concentration is not a concern. An absorbance assay is recommended for calibrating bovine serum albumin or other pure protein solutions for use as standards in other methods.

    Principle

    Proteins in solution absorb ultraviolet light with absorbance maxima at 280 and 200 nm. Amino acids with aromatic rings are the primary reason for the absorbance peak at 280 nm. Peptide bonds are primarily responsible for the peak at 200 nm. Secondary, tertiary, and quaternary structure all affect absorbance, therefore factors such as pH, ionic strength, etc. can alter the absorbance spectrum.

    Equipment

    In addition to standard liquid handling supplies a spectrophotometer with UV lamp and quartz cuvette are required.

    Procedure

    Carry out steps 1-4 (280 nm only) for a very rough estimate. Carry out all steps if nucleic acid contamination is likely.
    1. Warm up the UV lamp (about 15 min.)
    2. Adjust wavelength to 280 nm
    3. Calibrate to zero absorbance with buffer solution only
    4. Measure absorbance of the protein solution
    5. Adjust wavelength to 260 nm
    6. Calibrate to zero absorbance with buffer solution only
    7. Measure absorbance of the protein solution

    Analysis

    Unknown proteins or protein mixtures. Use the following formula to roughly estimate protein concentration. Path length for most spectrometers is 1 cm.

    Concentration (mg/ml) = Absorbance at 280 nm divided by path length (cm.)

    Pure protein of known absorbance coefficient. Use the following formula for a path length of 1 cm. Concentration is in mg/ml, %, or molarity depending on which type coefficient is used.

    concentration = Absorbance at 280 nm divided by absorbance coefficient

    To convert units, use these relationships:

    Mg protein/ml = % protein divided by 10 = molarity divided by protein molecular weight

    Unknowns with possible nucleic acid contamination. Use the following formula to estimate protein concentration:

    Concentration (mg/ml) = (1.55 x A280) – 0.76 x A260)

    Comments

    Cold solutions can fog up the cuvette, while warm solutions can release bubbles and interfere with the readings. For concentrated solutions (absorbance greater than 2) simply dilute the solution.

    Absorbance coefficients of some common protein standards:

    • Bovine serum albumin (BSA): 63
    • Bovine, human, or rabbit IgG: 138
    • Chicken ovalbumin: 70

    References

    • Layne, E. Spectrophotometric and Turbidimetric Methods for Measuring Proteins. Methods in Enzymology 3: 447-455. 1957.
    • Stoscheck, CM. Quantitation of Protein. Methods in Enzymology 182: 50-69. 1990.
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    Pages: Geri 1 2


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